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Structural, Electronic and Mechanical Properties of Re Doped FeMnP<SUB>0.67</SUB>A<SUB>0.33</SUB> (A=Ga and Ge): A DFT Study

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2022-11

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Kenya climate smart agriculture project (KCSAP)/world bank

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Science and Education publishing (SciEP)

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Chirchir, G. K., Mulwa, W. M., & Adetunji, B. I. (2022). Structural, Electronic and Mechanical Properties of Re Doped FeMnP<SUB>0.67</SUB>A<SUB>0.33</SUB> (A=Ga and Ge): A DFT Study. Science and Education Publishing (SciEP). https://repository.nrf.go.ke/handle/123456789/611

Abstract

The structural, electronic and mechanical properties of Re doped FeMnP0.67A0.33 (A= Ga and Ge) were examined by use of density functional theory (DFT) within the generalized gradient approximations as demonstrated in Quantum ESPRESSO code. The optimized structural parameters as well as derived lattice parameters are in consistent with other computational and achievable experimental results. The computed independent elastic constants confirm the mechanical stability of the investigated materials. The computed Poisson’s and Pugh’s ratios as well as Cauchy pressure, verify that FeMn0.67Re0.33P0.67Ga0.33 is the most ductile among the studied compounds. The calculated values of bulk modulus, shear modulus and Young’s modulus confirm high values of bond strength, hardness and stiffness of the investigated materials respectively. Therefore, the four compounds considered may be appropriate for industrial applications. The results report that FeMn0.67Re0.33P0.67Ga0.33 compound is more ductile and mechanically stable compared to other investigated compounds. This is the first qualitative computational prediction of the elastic properties of FeMnP0.67Ge0.33, FeMnP0.67Ga0.33, FeMn0.67Re0.33P0.67Ge0.33 and FeMn0.67Re0.33P0.67Ga0.33 compounds and this awaits experimental ratification. The calculated electronic density of states confirms that the Re_2p states are located in the conduction band (CB) in the unite cell while Re_3d dominate the CB in the supercell. Results from the doped compounds could not be compared with experimental or computational findings because to the best of our knowledge, this has not been done.

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Egerton University

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